Operando Optical Microscopy for Visualization of Dendrite Growth in an Argyrodite LPSCl-Polymer Composite Electrolyte

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dc.article.number104017
dc.article.number104017
dc.contributor.authorJin, Xiuyu
dc.contributor.authorHuang, Di
dc.contributor.authorMiao, Qiusu
dc.contributor.authorZhu, Ziting
dc.contributor.authorTong, Wei
dc.contributor.authorVidela Leiva, Álvaro Rodrigo
dc.contributor.authorLiu, Gao
dc.date.accessioned2025-05-01T10:32:55Z
dc.date.available2025-05-01T10:32:55Z
dc.date.issued2025
dc.description.abstractHerein, we demonstrate the utility of optical microscopy as an accessible technique for the in situ visualization of dendrite growth within polymer-sulfide composite solid-state electrolytes. The composite electrolyte features in situ polymerization and cross-linking of the polymer between ceramic particles, which opens up extensive opportunities for accelerated materials discovery, given the vast array of acrylate/methacrylate monomers available. Specifically, the cross-linked polymer poly(triethylene glycol dimethacrylate) (poly(TEGDMA)) was observed to effectively fill pores and inhibit dendrite growth at the lithium metal interface, attributed to its glassy state at room temperature. This work represents the first application of optical microscopy to illustrate that the incorporation of glassy, undoped polymers such as poly(TEGDMA) can serve as a viable strategy for dendrite suppression in solid-state composite electrolytes.
dc.description.funderU.S. Department of Energy
dc.description.funderLawrence Berkeley National Laboratory
dc.description.funderLDRD
dc.description.funderOffice of Science
dc.description.funderOffice of Basic Energy Sciences
dc.format.extent5 páginas
dc.fuente.origenScopus
dc.identifier.doi10.1021/acsenergylett.5c00281
dc.identifier.eisbn9780128194706
dc.identifier.eissn1878-5522
dc.identifier.isbn9780128231548
dc.identifier.issn2380-8195
dc.identifier.pubmedid36225231
dc.identifier.scieloidS0718-69242020000300109
dc.identifier.scopusidSCOPUS_ID:105001172836
dc.identifier.urihttps://doi.org/10.1021/acsenergylett.5c00281
dc.identifier.urihttps://repositorio.uc.cl/handle/11534/103922
dc.identifier.wosidWoS_ID: 001454190600001
dc.information.autorucEscuela de Ingeniería; Videla Leiva, Álvaro Rodrigo; 0000-0002-6785-5818; 10225
dc.issue.numero3
dc.language.isoen
dc.nota.accesoContenido completo
dc.pagina.final1957
dc.pagina.inicio1953
dc.publisherElsevier
dc.relation.ispartofPresent Knowledge in Food Safety: A Risk-Based Approach through the Food Chain
dc.revistaACS Energy Letters
dc.rightsacceso abierto
dc.subjectUgni molinae Turcz
dc.subjectUgni candollei Barm
dc.subjectGallic acid
dc.subjectCatechin
dc.subjectEutectic solvents
dc.subjectMicrowave-assisted extraction
dc.subjectNon-extractable polyphenols
dc.subject.ddc600
dc.subject.deweyTecnologíaes_ES
dc.subject.ods03 Good health and well-being
dc.subject.odspa03 Salud y bienestar
dc.titleOperando Optical Microscopy for Visualization of Dendrite Growth in an Argyrodite LPSCl-Polymer Composite Electrolyte
dc.typeartículo
dc.volumen10
sipa.codpersvinculados10225
sipa.indexScopus
sipa.trazabilidadCarga WOS-SCOPUS;01-05-2025
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