Operando Optical Microscopy for Visualization of Dendrite Growth in an Argyrodite LPSCl-Polymer Composite Electrolyte

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dc.catalogadorjlo
dc.contributor.authorJin, Xiuyu
dc.contributor.authorHuang, Di
dc.contributor.authorMiao, Qiusu
dc.contributor.authorZhu, Ziting
dc.contributor.authorTong, Wei
dc.contributor.authorVidela Leiva, Álvaro Rodrigo
dc.contributor.authorLiu, Gao
dc.date.accessioned2025-04-24T20:36:53Z
dc.date.available2025-04-24T20:36:53Z
dc.date.issued2025
dc.description.abstractHerein, we demonstrate the utility of optical microscopy as an accessible technique for the in situ visualization of dendrite growth within polymer-sulfide composite solid-state electrolytes. The composite electrolyte features in situ polymerization and cross-linking of the polymer between ceramic particles, which opens up extensive opportunities for accelerated materials discovery, given the vast array of acrylate/methacrylate monomers available. Specifically, the cross-linked polymer poly(triethylene glycol dimethacrylate) (poly(TEGDMA)) was observed to effectively fill pores and inhibit dendrite growth at the lithium metal interface, attributed to its glassy state at room temperature. This work represents the first application of optical microscopy to illustrate that the incorporation of glassy, undoped polymers such as poly(TEGDMA) can serve as a viable strategy for dendrite suppression in solid-state composite electrolytes.
dc.description.funderU.S. Department of Energy
dc.description.funderLawrence Berkeley National Laboratory
dc.description.funderLDRD
dc.description.funderOffice of Science
dc.description.funderOffice of Basic Energy Sciences
dc.fechaingreso.objetodigital2025-04-24
dc.format.extent5 páginas
dc.fuente.origenSCOPUS
dc.identifier.doi10.1021/acsenergylett.5c00281
dc.identifier.issn2380-8195
dc.identifier.scopusidSCOPUS_ID:105001172836
dc.identifier.urihttps://doi.org/10.1021/acsenergylett.5c00281
dc.identifier.urihttps://repositorio.uc.cl/handle/11534/103452
dc.information.autorucEscuela de Ingeniería; Videla Leiva, Álvaro Rodrigo; 0000-0002-6785-5818; 10225
dc.language.isoen
dc.nota.accesocontenido completo
dc.pagina.final1957
dc.pagina.inicio1953
dc.revistaACS Energy Letters
dc.rightsacceso abierto
dc.rights.licenseCC BY-NC-ND 4.0 Attribution-NonCommercial-NoDerivatives 4.0 International
dc.rights.urihttps://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subject.ddc600
dc.subject.deweyTecnologíaes_ES
dc.titleOperando Optical Microscopy for Visualization of Dendrite Growth in an Argyrodite LPSCl-Polymer Composite Electrolyte
dc.typeartículo
dc.volumen10
sipa.codpersvinculados10225
sipa.trazabilidadSCOPUS;2025-04-20
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